In cooperation with the Iranian Nuclear Society

Number of Volumes 39
Number of Issues 112
Number of Articles 1,263
Number of Contributors 2,672
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Number of Submissions 1,139
Acceptance Rate 29%
Time to Accept (Days) 92
Number of Indexing Databases 16
Number of Reviewers 892

Journal of Nuclear Science, Engineering and Technology (JONSAT) is an open access double-blind peer-reviewed publication. There is no charge for the article submission and article processing. Nuclear science and Technology Research Institute is the founder of the Journal and appoints the editorial boards. This journal is following of Committee on Publication Ethics (COPE) and complies with the highest ethical standards in accordance with ethical laws. All submitted manuscripts are checked for similarity through a trustworthy software (Hamyab) to be assured about its originality and then rigorously peer-reviewed by the international reviewers. (Read More...). 

Journal of Nuclear Science, Engineering and Technology succeeded in obtaining the "A" rank in the evaluation of scientific publications of the year 1402 by the Ministry of Science, Research and Technology.

This Journal is published in cooperation with the  Nuclear Society of Iran (NSI)

     

 

 

Calculation of the level density parameter and nuclear level density for 160-162Dy nuclei using the BCS model

Pages 1-10

https://doi.org/10.24200/nst.2024.1555.2012

Kh. Benam

Abstract Studying the structure of the nucleus through the consideration of pairing correlation between nucleons plays a crucial role in determining the thermodynamic properties of the nucleus. In this study, we examined the thermodynamic characteristics of the nucleus using the BCS model, which incorporates pairing correlation. The gap parameter serves as the symbol of pairing correlation in this model. By calculating the gap parameter at various temperatures using the BCS model, we were able to determine the excitation energy, temperature-dependent level density parameter, and nuclear level density. Additionally, we calculated the nuclear level density using the BSFG model and the temperature-dependent level density parameter. Finally, we compared the results of the nuclear level density obtained through these methods with each other and experimental data.

Investigating the effect of titanium atom doping on C3N monolayer

Pages 11-21

https://doi.org/10.24200/nst.2024.1568.2018

E. Cholaki; B. Arghavani Nia; S. Rezaee; S. Parsamehr

Abstract This article investigates the structural, electronic, optical, and thermoelectric properties of a titanium atom doped into a C3N monolayer using the Wien2K computational code and first principles calculations within the density functional theory framework. The study of electronic properties reveals metallic behavior in this two-dimensional structure. Optical properties demonstrate optical anisotropy in both the x and z directions. Analysis of the thermoelectric properties of the C3N@Ti single layer using the semi-classical Boltzmann theory indicates that this layer not only possesses a low Seebeck coefficient but also exhibits very small thermoelectric efficiency, limiting its thermoelectric application.

Determination of molybdenum in yellow cake by on-line solid phase extraction via homogenous sedimentation coupled to ICP-OES

Pages 22-29

https://doi.org/10.24200/nst.2024.1582.2024

S.R. Yousefi

Abstract In this study, an online homogenous sedimentation method was utilized for the in situ production of micro particles to be used as an adsorbent for solid-phase extraction of molybdenum. The process involved the dissolution of yellow cake and the conversion of molybdenum (VI) into a hydrophobic complex, followed by the addition of n-dodecyltrimethylammonium bromide as a precursor to the sample solution. A precipitant reagent, sodium hexafluoride, was then introduced into the solution through a T connection in a flow system. Micro particles were produced as a result of the interaction between the precursor and the precipitant reagent, which then adsorbed the molybdenum complex. After filtration, a desorption reagent was passed over the filter to release the adsorbed molybdenum, which was subsequently measured using ICP-OES. The method yielded a linear range of 0.2-200 µg/L, with a limit of detection of 0.05 µg/g. The repeatability of the method (RSD) was found to be 8.1% and 4.3% for concentrations of 10 and 100 µg/g, respectively. Overall, this method demonstrates potential for the precise and accurate determination of molybdenum in yellow cake samples.

Coating and characterization of Iodine-125 absorbent layer on the ferromagnetic core used in the Thermo-Brachytherapy system

Pages 30-38

https://doi.org/10.24200/nst.2024.1584.2025

E. Mohagheghpour; Sh. Sheibani; L. Farzin; R. Saber

Abstract A Ni-Cu (70.4-29.6 wt%) ferromagnetic alloy coated with an absorber layer of iodine-125 was used as the core in the Thermo-Brachytherapy (TB) system. The absorber layer, which was 100 μm thick and had a microcrystalline graphite structure, consisted of silver-doped activated carbon and polystyrene in a 70:30 weight ratio. Activated carbon is a preferred adsorbent for iodine capture due to its porous nature. Silver doping in the carbon enhances the trapping of iodine-125 through chemical adsorption. Polystyrene, acting as a binder in the absorptive layer's structure, facilitates the physical absorption of iodine on the surface of the silver-doped activated carbon-coated core. Results showed that the extraction efficiency of iodine-125 (as sodium iodide solution) with an average activity of 5 mCi on the nickel-copper core/polystyrene/silver-doped activated carbon was 20.31% after 2 hours. Coating the nickel-copper ferromagnetic core with gold or silver before depositing the silver-doped activated carbon increased the extraction efficiency to 32.77% and 60.23% after 2 hours, respectively. These findings highlight the significant impact of silver or gold coating on enhancing extraction efficiency. Moreover, a multi-step extraction process was employed in this research, where extraction steps were repeated to increase the recovery of iodine-125.

Determining the fuel assemblies bowing of the VVER-1000 reactor by using an artificial neural network and C-shape bowing assumption

Pages 39-48

https://doi.org/10.24200/nst.2023.1616

J. Vosoughi; N. Vosoughi; A.K. Salehi

Abstract FAs (Fuel Assembly) lateral deformation under mechanical, hydraulic, thermal, and radiation loads in the reactor core is called FA bowing. This phenomenon has different consequences for reactor safety and its operation. Bowing causes the local change in distance between the FAs, which leads to a neutron perturbation that affects the power distribution and its asymmetry. This research determines the bowing pattern of FAs in the VVER-1000 reactor core by using an artificial neural network and C-shape bowing assumption. That will be done based on power distribution caused by the presence of FA bowing. This issue will help the operator design the arrangement of FAs in the next cycle by knowing the bowing pattern in the reactor core. It will prevent the expansion of the bowing and its consequences in the next fuel cycles.

Investigation the fuel clad radiation damage by positron annihilation lifetime spectroscopy

Pages 49-58

https://doi.org/10.24200/nst.2024.1637

R. Jafari; M.A. Amirkhani Dehkordi; E. Yahaghi; B. Rokrok; M. Asadi Asad Abad

Abstract Identification of the changes of aluminum structure due to neutron radiation is very important in the reactor fuel clad. In some cases, ion (usually proton beam) irradiation method is implemented for this investigation. The changes in the holes of Al are in the range of picometers by the radiation of energetic protons. In this research, positron annihilation lifetime spectroscopy, was used to investigate the changes of holes in Al-6061 and Al-303 due to the radiation of 2.2 MeV protons at different amounts of radiation. This method has the ability to evaluate the dimensions of the holes in the range of picometers and nanometers. For both investigated aluminum samples, the results show that the value of τave first decreased and then increased. It indicates the holes became smaller and decrease the vacancy defects in the initial stages of irradiation. Then, the holes became larger in the continuation of irradiation, which indicates increasingin the interstitial defects. These results were also confirmed by XRD test. It can be seen that the crystal size of the irradiated aluminum increased at the in the initial stages of irradiation and then decreased in the continuation of irradiation.

Neutronics and shielding simulation and evaluation of a second pool of a typical research reactor as spent fuel pool

Pages 59-67

https://doi.org/10.24200/nst.2024.1641

E. Boustani; M. Hasanzadeh

Abstract The design calculations of the spent fuel pool require the consideration of various parameters such as neutronic, thermal-hydraulic, safety, shielding, economic and operation. Considering the high cost of designing and building of a new spent fuel pool as well as the existence of empty spaces in the pool of some research reactors, neutronic and shielding calculations for the feasibility of using second pool of a typical research reactor as a spent fuel pool is done using ORIGEN2.1 and MCNP6 codes. The first step is the determination of the distance between fuels (grid pitch) in such a way that the effective multiplication factor for the worst possible case is less than 0.95, that 13 cm grid pitch fulfills this condition. Source term calculation for a fuel with the highest burnup (60%) is done as the most pessimistic condition. Continuous operation and 24 hours cooling are considered as the shortest possible time to transfer spent fuels to the storage rack in order to have the most pessimistic conditions in the design of spent fuel rack. For a rack with 100 spent fuels that is 87 cm away from the pool wall on each side, a 300 cm layer of water on top of the fuels and 85 cm thick concrete wall are enough for the possibility of using second pool as a spent fuel pool. It has been found that it meets the dose rate criteria of less than 1 and 10 μSv/h behind the wall and above the pool water level.

Extension of mixed of symmetries method in the calculation of electric quadrupole transition rate of Cadmium isotopic chain

Pages 68-78

https://doi.org/10.24200/nst.2024.1521.1991

H. Sabri; A.R. Jabbari; M. Sayedi

Abstract In this paper, in the framework of the interacting boson model (IBM), the method of mixed U(5) and SO(6) symmetry limits has been used to calculate the electric quadrupole transition rates between different levels in the isotopic chain of Cadmium (110-104Cd) and in the E < 3 MeV region. In this method, wave functions of different intruder levels are considered as a combination of wave functions in the two N and N+2 bosons spaces and the effect of electric quadrupole transition's operator is determined by them. The effective charges of the transition operator are extracted in comparison with the experimental values of the quadrupole transition rates and then, theoretical predictions of two methods, using only U(5) dynamical limit and mixed of symmetries are compared with each other. The results show that the accuracy of the predictions are increased via mixed of symmetries method in all of considered transitions. On the other hand, the U(5) dynamical limit is only successful in examining the quadrupole transitions between the levels of the ground band and levels with a longer half-life and confirms the existence of a closed neutron sub-shell in the 106Cd nucleus. Also, for such inter-bands transition and also transitions are originated from intruder states, the exactness of the mixed symmetries prediction are obvious.

Qualitative and quantitative determination of technetium-99 in the concentrated waste of Bushehr nuclear power plant

Pages 79-88

https://doi.org/10.24200/nst.2024.1649

R. Yavari; K. Saberian; A. Maleki Farsani; B. Salimi; B. Soleimanzade; A. Heydari; M. Tabasi

Abstract Technetium-99 in nuclear waste as one of the toxic and hazardous radioactive pollutants should be quantitatively and qualitatively identified before final disposal. In the present research work, Technetium -99 in the aqueous phase of the concentrated waste of Bushehr nuclear power plant was qualified and quantified. To achieve this goal, Cesium-134 and 137 were firstly separated using potassium cobalt hexacyanoferrate(II) adsorbent. Then, tritium was removed using thermal treatment at 60˚C, and finally technetium-99 in this media was purified by removing beta emitter radioisotopes such as cobalt- 60, iron-55, and nickel-63 using precipitation process with iron(III) hydroxide. The samples were qualitatively and quantitatively evaluated using gamma spectrometry and liquid scintillation counter instruments. The results showed that purified Technetium-99 has a high radiochemical purity and other radioisotopes were removed from the media with an efficiency of about 100%. Also, the beta spectrum of the sample was in complete accordance with the beta spectrum of the standard samples. The total yield of the proposed processes using the increase of Technetium-99m tracer to the original sample was equivalent to 80.69%. Taking into account the 93% efficiency of the liquid scintillation counter and the processes yield (80.69%), the specific activity of Technetium-99 was calculated as 10554.13 Bq.L-1.

Uranium extraction and production of yellow cake from phosphoric acid using solvents D2EHPA and TRPO

Pages 89-97

https://doi.org/10.24200/nst.2024.1548.2010

D. Ghoddocy Nejad; H. Zare Tavakoli; R. Roshani; A.H. Kiarashi

Abstract In this research, uranium extraction from a phosphoric acid solution produced from a new phosphate ore from a Syrian mine was carried out for the first time using D2EHPA-TRPO solvents in kerosene. The goal of the research was to produce yellowcake from the phosphoric acid solution. The process involved primary solvent extraction, primary stripping, secondary solvent extraction, scrubbing, and finally secondary stripping with precipitation. Based on the results obtained, the optimal values for primary solvent extraction factors were: O/A ratio of 1/3, temperature of 40°C, mixing time of 7 minutes, and TRPO concentration of 6% (v/v). The optimal values for primary stripping factors were: O/A ratio of 34/1 (two steps with O/A ratio of 17/1), temperature of 40°C, and mixing time of 40 minutes. The efficiency of these two processes was 86.40% and 95.60%, respectively. The optimal conditions for the secondary solvent extraction process included an O/A ratio of 1/4, temperature of 40°C, and mixing time of 7 minutes. For scrubbing the charged solvent with sulfuric acid (w/v), 2.5% of the optimal values of O/A ratio of 10/1, temperature of 40°C, and mixing time of 7 minutes were used. Finally, for secondary stripping and precipitation of yellowcake, a 2M solution of ammonium carbonate was used at a temperature of 40°C, and the stirring time was 15 minutes.

An investigation of deep learning techniques for automatic pelvic CT scan segmentation

Pages 98-108

https://doi.org/10.24200/nst.2024.1585.2026

E. Ghaedi; A. Asadi; S.A. Hosseini; H. Arabi

Abstract Radiotherapy treatment planning requires accurate delineation of organs at risk (OAR), which is typically a manual and time-consuming process. This research aims to explore the feasibility of using deep learning algorithms as an automatic tool for segmenting CT scan images. Accordingly, the performance of several convolutional neural networks (CNNs), including U-Net, Residual U-Net, and SegResNet, was compared as tools for automatic segmentation of OARs in pelvic CT scans (bladder, prostate, rectum, left femoral head, and right femoral head) against manual segmentation by specialists. This study involved 238 patients for prostate segmentation and 218 patients for the other four organs. The models' performance was assessed using metrics such as the Dice similarity coefficient, Jaccard index, and Hausdorff distance. The SegResNet model, providing the best performance, achieved Dice coefficients of 0.956, 0.832, 0.864, 0.980, and 0.985 for the bladder, prostate, rectum, left femoral head, and right femoral head, respectively. In summary, the results indicate that convolutional neural networks can accurately segment organs at risk in radiotherapy planning, with accuracies above 95% for bones and bladder, and over 83% for the rectum and prostate, while also speeding up the segmentation process.

Simulation and design of disc-type beam-shaping assembly for X-ray back scatter whole-body imaging system

Pages 109-122

https://doi.org/10.24200/nst.2024.1592.2029

Z. Alipour; M.R. Pahlavani

Abstract The X-ray backscatter imaging systems have unique inspection capabilities and practical features due to their high sensitivity to organic materials, low radiation dose, and ability to scan from one side of the object. The scan is performed by an X-ray pencil beam. The shape, size, and intensity of the beam play a significant role in the image quality and the radiation dose received by the person. To create a pencil-shaped beam, the cone-shaped beam of the X-ray tube passes through a fan beam collimator and a chopper wheel. Different designs were simulated to optimize the fan beam collimator and chopper wheel, considering factors such as length and gap of the collimator, as well as the slit width of the disc using the MCNPX2.6 code. To minimize leakage dose, a 4-mm tungsten/copper alloy disc was determined to be the most suitable in terms of thickness and material. Based on the simulation results from image quality tests, it was found that a collimator with a length of 20 cm, a 1 mm gap, and a 1 mm slit width of the disc produced the most optimal X-ray beam for backscatter whole-body imaging systems. The best image quality was achieved at a disc rotational speed of 1500 rpm and a relative speed of vertical movement at 40 cm/s.

Mineralogical studies of uranyl minerals with field emission electron microscope in the Khoshoumi Anomaly 6 deposit (Block 1), Bafq-Saghand metallogenic belt

Pages 123-134

https://doi.org/10.24200/nst.2024.1594.2030

Kh. Khoshnoodi; S. Ziapour

Abstract Khoshoumi Anomaly 6 is a significant uranium deposit located in the Bafq-Saghand metallogenic belt within the Central Iran zone. The gneiss serves as the primary host for uranium mineralization in block 1 of Khoshoumi Anomaly 6. Field emission electron microscopy studies have identified two stages of uranium mineralization within the area: primary mineralization (hypogene) and uranyl silicate (supergene). Primary uranium minerals found in the hypogene zone include uraninite, with minor amounts of thorouraninite, brannerite, and uranothorite. Uranyl silicate mineralization is observed along fractures in the form of boltwoodite and soddyite. Over time, boltwoodite undergoes alteration into sodium-boltwoodite and uranophane. Field evidence and mineralogical studies suggest that meteoric fluids, with a neutral to alkaline pH and low temperature, played a role in leaching uranium, silicon, potassium, sodium, and calcium from the gneiss. These elements were then deposited along fractures as uranyl silicate minerals, accompanied by calcite, clay, and chlorite. The presence of calcite alongside uranyl silicates indicates the transport of uranium in the form of uranyl carbonate complexes within the fluid.

Electron beam control in the storage ring of the ELETTRA 2.0 accelerator using machine learning

Pages 135-147

https://doi.org/10.24200/nst.2024.1598.2034

M.S. Yazdani; S.F. Masoudi; J. ًRahighi; S. Dastan

Abstract In recent years, the advancement of electron synchrotron light sources has been crucial for synchrotron radiation users. Improving electron beam qualities, such as stability and intensity, has been key to generating high-brightness photon beams. To achieve a brighter photon beam, electron synchrotron accelerators have been undergoing significant design changes. A critical aspect of their design is precise control of particle trajectories and correction of errors to achieve a stable electron beam and, consequently, a high-intensity photon beam. One interesting approach in this field is the use of neural networks to correct the electron beam position in the storage ring, a process known as beam control. In this study, a convolutional neural network model has been developed for the first time to control the ELETTRA 2.0 storage ring, a synchrotron light source in Italy. The performance of this model, based on machine learning techniques, is approximately 6% better than the ISVD method, while also demonstrating high robustness to real-world data.

Optimization of molecular pump by meta-heuristic algorithms: modified Sickafus method

Pages 148-159

https://doi.org/10.24200/nst.2024.1604.2038

M. Khajenoori; S. Yousefi-Nasab; S.J. Safdari; S. Basiri

Abstract It is important to maintain the vacuum in the space between the rotor and the body of a gas centrifuge machine during the gasification and enrichment process. For this reason, a molecular pump is connected to the upper part of the body. The pump has grooved that particles collide with as they move. Depending on the direction of the grooves, the particles are deflected and return to the rotor. One method of analyzing the gas flow inside the molecular pump is by solving the flow equations using the Sickafus method and his colleagues. This method is useful because it reduces calculation time. In this article, four meta-heuristic algorithms were used to determine the optimal geometric and operational parameters of the molecular pump. The results indicate that among the meta-heuristic algorithms, optimization with the humpback whale algorithm (WOA) produces the highest compression ratio for the molecular pump. The average absolute deviation value of the logarithm of the pressure density ratio, when compared to values predicted by the upgraded Sickafus method with optimal parameters, shows a very good agreement between the experimental method and the upgraded Sickafus method using the meta-heuristic WOA algorithm.

Production and quality control of the 132/135La theranostic pair for targeted radiotherapy

Pages 160-169

https://doi.org/10.24200/nst.2024.1646.2045

A. Shirpoor; A. Haddadi; S. Zolghadri; S. Vosoughi; S. Rajabifar

Abstract Among promising radioisotopes, 132/135La stands out as a theranostic pair, offering specific advantages for the preparation of a wide range of radiopharmaceuticals. In this study, the theranostic pair 132/135La was produced through the interaction of natBa(p,x)13xLa, using theoretical calculations with the nuclear codes ALICE-91, TALYS-1.8, and SRIM-2013. The natural barium target was then irradiated in a 30 MeV cyclotron with 22.5 MeV protons and a current of 100 μAh. After the lanthanum was separated from the irradiated target, the solution's chemical purity, radiochemical purity, and radionuclide purity were examined using ICP-OES, RTLC, and gamma spectrometry, respectively. The study also investigated the effect of increasing the concentration of the chelator DOTA (1-100 nanomolar) on its labeling with lanthanum. The results showed that the average total amount of metal ions in the final solution was less than 0.1 ppm, with radiochemical and radionuclide purities above 99% and 99.5%, respectively. The labeling of the chelator DOTA with lanthanum demonstrated that even with the addition of 1 nmol of this chelator, a radiochemical purity higher than 93% was achieved. This study indicates that it is possible to produce lanthanum radionuclides with the required quality for the development of theranostic radiopharmaceuticals.

Investigating the effective parameters on the recovery of rare earth elements from Chahgaz ore using acid washing process

Pages 170-178

https://doi.org/10.24200/nst.2024.1655.2048

M. Rezaee

Abstract   In this research, the recovery of rare earth elements from Chahgaz ore has been investigated through an acid leaching process. The effect of different parameters on the dissolution of rare earth elements was also explored. The results indicated that factors such as acid concentration, leaching temperature, ore particle size, liquid to solid ratio, and leaching time are crucial in recovering rare earth elements from the ore. Specifically, the recovery percentage of rare earth elements in sulfuric acid was found to be higher compared to other acids. Increasing the temperature to 85 degrees Celsius was observed to accelerate the leaching reaction and enhance the recovery of rare earth elements. Moreover, increasing the liquid to solid ratio up to 2 led to improved contact between the solid and liquid phases, as excess acid in the reaction medium facilitated a higher leaching rate of rare earth elements. Optimal conditions for the leaching process were determined to be a temperature of 85 degrees Celsius, a leaching time of 6 hours, a sulfuric acid concentration of 1.5 M, a liquid to solid ratio of 2, and a particle size of 150 microns. Under these conditions, a recovery percentage of 95% for rare earth elements from Chahgaz ore was achieved.

Comparison of filtering fast neutrons by externally-purchased sapphire crystal (plane 112) and home-made Iranian sapphire crystal (plane 111)

Pages 179-189

https://doi.org/10.24200/nst.2024.1665.2051

Z. Gholamzadeh; R. Ebrahimzadeh; S. Shamaleki; A. Biganeh; H. Saebi

Abstract Neutron filter crystals are widely used in the nuclear industry, particularly in research reactors. One of the most important crystals used is sapphire crystal, which is grown in several countries to ensure good quality. This research aims to compare the neutron performance of sapphire crystals made in Iran with those of externally supplied crystals. An Am-Be source was used in this study to assess the ability of these sapphire crystals to remove fast neutrons. Additionally, a monochromatic neutron beam was used to study the impact of these crystals on reducing the intensity of the neutron flux. To verify the accuracy of computational codes in simulating the neutron behavior of these filter crystals, the McStas code was utilized. The results of this simulation were then compared with available experimental data. Comparing the experimental results with those published worldwide revealed that the domestically grown crystals performed comparably to the foreign samples. The experimental findings showed that a 2.5 cm sapphire crystal filtered the monochromatic neutron beam with an energy of 0.06 eV by only about 5.5%, and fast neutrons with an energy of more than 200 keV by about 33%. Increasing the crystal thickness to approximately 6 cm increased the filtration of fast neutrons to about 60% and monochromatic neutrons to about 16.5%. Overall, the results of this study indicated that the discrepancies between the simulation and experimental values may be attributed to the lack of detailed information necessary for crystal modeling in the computational code.

Estimation of radiation dose in the upgraded Damavand tokamak and the design of safe radiation shielding

Pages 190-197

https://doi.org/10.24200/nst.2024.1672.2055

S. Yarmahmoodi; B. Pourshahab; Ch. Rasouli

Abstract Tokamaks are recognized as one of the most promising devices for achieving nuclear fusion, operating within complex environments with high radiation levels. Upgrading these devices to enhance plasma efficiency and duration inevitably leads to increased radiation levels, making precise radiation dose estimation and the design of effective shielding systems essential. The Damavand tokamak, with its pure hydrogen plasma, generates both soft and hard X-rays. With sufficient data on these indirect ionizing radiations, the potential adverse effects can be minimized. Planned upgrades to the Damavand tokamak will extend plasma pulse duration from 22 ms to approximately 200 ms, resulting in a significant increase in radiation levels, estimated to be up to ten times higher in work areas, posing safety risks for personnel. In this study, we estimate the radiation dose in different areas of the upgraded Damavand tokamak laboratory based on experimental data, and we calculate specifications for new radiation shields using the MCNPX code to ensure laboratory safety. The required shielding dimensions were calculated for lead and concrete materials, allowing for a cost and feasibility assessment to guide the selection of the optimal implementation material.

The effect of pre-ionization on improving the performance of mather type plasma focus device MTPF2.4kj

Pages 198-206

https://doi.org/10.24200/nst.2024.1579.2022

S. Fazelpour; A. Chakhmachi; A. Nasiri

Abstract The impact of pre-ionization using a 330 MΩ shunt resistor on the performance characteristics of a Mather Type plasma focus device with 2.4 kJ of energy, charged by a 12 μF capacitor bank to a maximum voltage of 20 kV, will be discussed in relation to hydrogen gas. In this study, the signal characteristics of the current and the current derivative of the device were measured and compared with and without pre-ionization at an optimal operational pressure of 0.85 Torr. Additionally, the emitted hard X-rays and ion beam in each shot were measured using a Ne102 X-ray plastic scintillation detector and Faraday cup, respectively. These measurements were conducted and compared with and without pre-ionization at the optimal pressure. The results from the current and current derivative signals of the device indicate that with initial pre-ionization, the signals exhibit a deeper and sharper fracture at the pinch time compared to when the pre-ionization circuit is inactive. This suggests that a stronger and more defined pinch occurs with pre-ionization. Furthermore, analysis of the Faraday cup signal amplitudes reveals that the intensity of emitted hard X-rays is significantly higher when pre-ionization is utilized compared to when it is not. Therefore, pre-ionization markedly enhances the efficiency of the plasma focus device, increases the intensity of emitted hard X-rays, and generates an ion beam with a higher current.

NUCLEAR FUEL CYCLE AND FUEL MATERIALS

Study of mass transfer parameters and identification of rate-controlling step in the cerium and yttrium ion exchange process in a fixed bed column

Articles in Press, Accepted Manuscript, Available Online from 07 June 2025

https://doi.org/10.24200/nst.2025.1797.2108

Amin Ildarabadi; Maryam Khajenoori; Fazel Zahakifar; Ahmad Ghadiri

Abstract In this study, the ion exchange process of cerium and yttrium using Dowex 50W-X8 resin was investigated and the behavior of the breakthrough curves were reported. The ion exchange percentage for Ce(III) and Y(III) was 73.93% and 70%, respectively. Mathematical modeling was performed to calculate the mass transfer components. Various mass transfer resistance mechanisms such as film diffusion resistance, intraparticle diffusion and axial dispersion as well as other mass transfer approximations were investigated by the linear driving force (LDF) model. Investigations showed that intraparticle diffusion resistance had the largest contribution in the ion exchange process of rare elements cerium and yttrium (R_f<R_ax<R_int). Intraparticle diffusion, i.e. the second stage of the overall ion exchange mechanism, was identified as the controlling stage of the process. Also, the Biot number for Ce(III) and Y(III) was greater than 30, indicating that the rate-controlling step of the ion exchange process was intraparticle diffusion. Thus, the accuracy of the studies was confirmed. The Peclet number also matched the slope of the breakthrough curves well.

GENERAL AND MISCELLANEOUS

Preparation,, Quality Control and Biodistribution of 123I-MIBG

Articles in Press, Accepted Manuscript, Available Online from 10 June 2025

https://doi.org/10.24200/nst.2025.1796.2106

Mohammad Mirzaei; Saeed rajabifar; mohammad Rahimi; Somayeh Rasouli Garmarodi; Hasan Yousefnia

Abstract Iodine-123 radionuclide was produced through the bombardment of a xenon-124 gas target using protons with energy of 28.5 MeV in a cyclotron accelerator. After confirming the quality control procedures, the iodine-123 radionuclide with a purity of more than 99% and activity concentration of 8.47 ± 0.2 GBq/mL was used for labeling of MIBG chemical compound. The quality control of the labeled compound was performed using thin layer chromatography method by acetic acid:water:butanol (1:1:4) as the mobile phase. The quality control results indicated a radiochemical purity of more than 99% for the final product. The biodistribution of the radiolabeled compound was evaluated following the injection of 5.5–11.1 MBq of the 123I-MIBG radiopharmaceutical into rats, and the rats were dissected at various time intervals and imaging was performed. A comparative analysis of the biodistribution of free 123I and 123I-MIBG revealed that the radiolabeled compound exhibited a distinctly different biodistribution pattern compared to free 123I.

RADIOLOGY AND NUCLEAR MEDICINE

Accurate diagnosis of primary and metastatic brain tumors using laser fluorescence imaging guided by the sodium fluorescein exogenous fluorophore

Articles in Press, Accepted Manuscript, Available Online from 09 July 2025

https://doi.org/10.24200/nst.2025.1768.2090

Fatemeh Ghoghaii; Maryam Ilchi-Ghazaani; Mahsa Ghezelbash; Batool Sajad

Abstract In this study, the accurate diagnosis and differentiation of healthy and cancerous brain tissues was investigated using laser fluorescence imaging guided by the sodium fluorescein exogenous fluorophore and the results are compared with tissues auto-fluorescence images. Samples, which were diagnosed as meningioma, metastatic carcinoma, low-grade glioma, as well as high-grade glioma types by pathologists, were obtained from 4 patients and optical imaging technique with hematoxylin-eosin staining is used to validate the results. The findings reveal that the intensity of fluorescence radiation from cancerous tissues is more intense than that from healthy tissues due to the greater permeability of the dye in the cavities and pores of the tissue. In addition to increasing the accuracy and precision of the results, this imaging method allows the surgeon to visualize and diagnose the tumor in real-time and completely resect the tumor, eliminating the need for invasive biopsies. Therefore, the results indicate that sodium fluorescein can be used as a reliable fluorescence marker in intraoperative imaging to improve the diagnosis and delineation of brain tumors.

SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS

Experimental Analysis and Numerical Simulation of Boiling Heat Transfer Process on Surfaces with Varying Wettability Properties

Articles in Press, Accepted Manuscript, Available Online from 06 May 2025

https://doi.org/10.24200/nst.2025.1759.2087

Aref Rahimian

Abstract An anodic electrophoretic method has been used to create a uniform thin film coating on thin steel plates. The changes in the contact angle of the plates have been carefully measured. Then the samples were tested in a boiling pool to measure the critical heat flux and the boiling heat transfer coefficient. For the numerical simulation of plates with different wettability, after validation, by changing some of the boiling parameters to parameters that depend on the contact angle, the critical heat flux has been calculated for variable contact angles. The experimental results and numerical simulation are close to each other and show a similar trend. These results are also compared with other experimental data and their difference is less than 5%.

MATERIALS SCIENCE

The influence of hot rolling-induced microstructural changes on the mechanical properties and fracture behavior of homogenized Ni-12.5Mo-7.8Cr nickel-base superalloy

Articles in Press, Accepted Manuscript, Available Online from 05 May 2025

https://doi.org/10.24200/nst.2025.1758.2086

Morteza Sarvarilale; Sorosh Bakhshi

Abstract Nickel-based alloys were highly regarded due to their strength and good corrosion resistance at high temperatures. From the group of nickel-based superalloys, the Ni-12.5Mo-7.8Cr alloy has attracted the attention of researchers more than other structural materials due to its low production cost, easy access, excellent weldability, and excellent resistance to hot corrosion. In this research, the microstructural changes caused by hot rolling on the mechanical properties and fracture behavior of Ni-12.5Mo-7.8Cr nickel base superalloy were studied and investigated. For this purpose, hot rolling operation at 1100 °C was performed on the homogenized ingot at 1177 °C for 20 minutes. Microstructural investigations, fracture behavior and mechanical properties were carried out using optical and electron imaging analyzes and tensile tests. Microstructural investigations showed the formation of coarse and fine grains and creation of inhomogeneous structure after the hot rolling process. Also, according to the tensile test results, hot rolling led to an improvement of approximately 120% yield strength and a decrease of approximately 13% in the final tensile strength. Also, the fracture pattern of the homogenized and rolled sample shows the change of the fracture mechanism from soft to grain boundary brittle as a result of hot rolling.

RADIOLOGY AND NUCLEAR MEDICINE

Analysis and Evaluation of Oxygen-18 Isotope Separation via Cryogenic Distillation Using MATLAB Software

Articles in Press, Accepted Manuscript, Available Online from 15 March 2025

https://doi.org/10.24200/nst.2025.1743.2081

Hedieh Ahmadi; Mohammad Rahgoshay; Amir Heidarynasab

Abstract Positron Emission Tomography (PET) is an advanced tool for the diagnosis and staging of cancer, based on the detection of glycolytic activity in malignant cells. This method requires drugs such as Fluorine Deoxy Glucose (FDG), the production of which necessitates the separation of Fluorine-18 and Oxygen-18 isotopes with a purity exceeding 95%. The use of cryogenic distillation columns as a suitable method for producing enriched oxygen is significant, despite the associated challenges of cost and efficiency. This study investigates the optimization of distillation column performance, analyzing the effects of factors such as input temperature and pipe height using MATLAB software. The results indicate that the maximum separation of the desired isotope depends on the type of isotope and the conditions of the apparatus, while the type of feed has no effect on concentration distribution. These findings can contribute to the development of optimization methods for the production of isotopes needed in medical imaging.

GENERAL AND MISCELLANEOUS

Evaluation of Natural Ventilation Efficiency in Reducing Radon Concentration in an Apartment Unit Using Computational Fluid Dynamics (CFD)

Articles in Press, Accepted Manuscript, Available Online from 05 April 2025

https://doi.org/10.24200/nst.2025.1721.2071

B. Azarvand-Hassanfard; M. Gholami

Abstract The radioactive radon gas infiltrates enclosed spaces through building materials and soil, and its accumulation in buildings with inadequate ventilation can pose health risks to residents. This study simulates and analyzes the impact of ventilation rates and building interior geometry on airflow patterns and radon distribution in an apartment unit using Computational Fluid Dynamics (CFD). The simulation results showed that the behavior of airflow and radon accumulation under various ventilation rates cannot be precisely predicted. Despite a reduction in average radon concentration due to increased ventilation rates, localized radon buildup occurs in certain areas due to vortex flows, with concentrations in these spots reaching multiple times the average concentration. These findings highlight the limitations of natural ventilation in creating a stable and uniform flow pattern for the complete removal of radon from all areas within the interior space. Additionally, a comparison of simulation data with experimental measurements showed a good match, confirming the accuracy of the CFD model. The findings of this study indicate that to effectively reduce radon concentration in enclosed spaces, precise ventilation system design that considers airflow patterns and the complexities of spatial geometry is essential.

OTHER INSTRUMENTATION

Proton path tracking in proton computed tomography using machine learning.

Articles in Press, Accepted Manuscript, Available Online from 12 January 2025

https://doi.org/10.24200/nst.2025.1719.2070

zohreh ramezani; zafar riazi; Naser vosoughi; Ehsan Alibeigi

Abstract One of the main problems in proton computed tomography is the reduction of the spatial resolution of the image due to the multiple coulomb scattering of protons while passing through the material. To deal with this problem, it is necessary to model the most likely path of protons (MLP). In this regard, artificial neural networks, as one of the innovative solutions in the field of machine learning, have helped to improve the accuracy of estimating the most likely path of protons. In this study, an artificial neural network with adaptive moment estimation optimization algorithm was designed to estimate the most likely proton path (MLP). The training of the network was done using the data obtained from the simulation of the proton computed tomography system in Geant4, so that 60% of this data was allocated for training, 20% of the data for validation, and 20% for the model test. These data contained information such as the position of entry and exit of protons, energy deposit, exit angle of protons and 10 points forming the path for each proton. The image matrix was modified with the help of the most likely path estimated by the neural network (MLP) and the cubic spline path (CSP), and the image was reconstructed using the Filtered Back Projection algorithm. The results of this study showed that the MLP method was able to achieve a spatial resolution of 5 line pairs/cm, while this value was equal to 3 line pairs/cm for the CSP method.

PARTICLE ACCELERATORS

ASE derived Shock wave propagation in the laser-driven ion acceleration mechanism

Articles in Press, Accepted Manuscript, Available Online from 01 January 2025

https://doi.org/10.24200/nst.2025.1717.2069

mohammad jafar jafari; somayeh rezaei

Abstract The Target Normal Sheath Acceleration (TNSA) method is one of the most efficient techniques for laser ion acceleration. One of the main challenges in optimizing this method is the detrimental impact of laser pre-pulses on the target, which can lead to plasma formation and changes in material density and temperature, resulting in shock wave formation and reduced acceleration efficiency. This study investigates the effects of laser pre-pulse duration and intensity (ASE) and target material on the formation and propagation of shock waves in the proton acceleration process via the TNSA method. The numerical results and one-dimensional hydrodynamic simulations indicate that, at lower ASE intensities (around 1011 W/cm2 and durations of 1 to 2 nanoseconds), the aluminum foil target undergoes minimal displacement, and due to the lack of deformation at the target’s rear side, It is expected that due to the lack of deformation at the target’s rear side, ion acceleration performance will not degrade. However, as the pre-pulse intensity increases, especially in lighter materials such as CH polymer, density variations and target displacement become more pronounced, which reduces the acceleration efficiency. These findings provide a basis for determining optimal conditions for laser acceleration experiments.

PLASMA PHYSICS AND FUSION THECHNOLOGY

Design and Construction of the Laser Facility for Studying Inertial Confinement Fusion

Articles in Press, Accepted Manuscript, Available Online from 14 July 2025

https://doi.org/10.24200/nst.2025.1712.2068

Amir Hossein Farahbod; H. Farokhi; M. Masoudi Ghazyar; M. Pishdast; M. Taheri; H. Movahedinejad; M.S. Mamduhe; S.M. Zahedi-Dizaje; R. Sabre; M. Jaberi; S.A. Ghaseme; M.R. Jafari Milani; N. Morshedian; A. Momeni; H. Ghasemi; A.R. Farzane Goradel; K. Asgari Deylame; R. Nourian; N. Ardalani; A. Khalilzade

Abstract In this article, the structure and performance of the designed and constructed laser facility to perform basic research on the field of inertial confinement fusion and laser-plasma interaction have been studied. The laser facility has four laser beams and the optical amplifiers are based on the phosphate Nd:Glass solid-state active medium. The vacuum spatial filters have improved the beam quality and reduced the misalignment sensitivity of the optical structure. More than 30 Joules per beam have been achieved, and the total optical energy of the laser facility exceeds 120 J. The laser facility is upgraded to increase laser optical energy to 500 J. Temporal pulse-shaping of the laser master oscillator, the optical self-alignment systems, and equalization of the propagation time of laser beams from the laser source to the target position based on the heterodyne interferometer, are the main activities to make the implosion experiments of the pellets filled with the heavy isotopes of hydrogen for studying the inertial confinement fusion.

PARTICLE ACCELERATORS

Effect of the laser pulse shape on the ionization-induced trapping of electrons in laser-plasma accelerators

Articles in Press, Accepted Manuscript, Available Online from 21 December 2024

https://doi.org/10.24200/nst.2024.1689.2061

Elnaz Khalilzadeh; amir chakhmachi; zohreh dehghni

Abstract In this paper, the injection of Nitrogen electrons due to ionization in a laser-plasma accelerator is studied. For this purpose, the propagation of short and intense laser pulses with different pulse shapes in a combination of Hydrogen atoms (low atomic number) and Nitrogen atoms (high atomic number) is considered. Using the single-particle Hamiltonian in the plasma wave field caused by the ionization of Hydrogen atoms, the physics and the mechanism of electron ionization injection in the appropriate phase are investigated. Then, the results of the particle-in-cell (PIC) simulation code show that the population and maximum energy of the trapped and injected nitrogen electrons due to ionization are strongly dependent on the laser pulse shape.

NUCLEAR DISARMAMENT, SAFEGUARDS AND PHYSICAL PROTECTION

Intelligent Surveillance System for Real-Time Radioactive Materials Localization and Identification Based on Fusion of Vision and Radioactive Spectroscopy

Articles in Press, Accepted Manuscript, Available Online from 09 July 2025

https://doi.org/10.24200/nst.2025.1687.2060

Hadi Ardiny; AmirMohammad Beigzadeh

Abstract This research presents an innovative surveillance system capable of real-time detection, identification, and localization of radioactive materials within video feeds from surveillance cameras. By combining advanced image processing algorithms and gamma-ray spectroscopy, this system offers a novel approach to the challenge of radioactive material detection. Image processing techniques are employed to identify and track objects, such as bags or packages, that may contain radioactive materials. Simultaneously, gamma-ray spectrometers measure the energy spectra emitted by radioactive sources, enabling the identification of radionuclides through spectral analysis. Data fusion techniques integrate the information derived from image processing and spectroscopy, yielding accurate and reliable localization and identification of radioactive materials. Experimental results demonstrate that detector placement and distance from the radioactive source significantly influence the system's performance. In a recent experiment, the system identified and localized a contaminated radioactive source containing Cs-137 (100 ci) within 20 seconds and 5 seconds, respectively. This approach offers a cost-effective and efficient solution for radioactive material detection and localization, surpassing conventional methods. With broad applications in world security, nuclear facility monitoring, and environmental surveillance, this innovative system empowers timely and informed decision-making in the face of nuclear threats and incidents, enhancing preparedness and response capabilities.

NUCLEAR FUEL CYCLE AND FUEL MATERIALS

Investigating effective of parameters and kinetic model of uranium absorption from uranium containing solution by ion exchange resin

Articles in Press, Accepted Manuscript, Available Online from 21 October 2024

https://doi.org/10.24200/nst.2024.1679.2057

davood ghoddocy nejad

Abstract In this research, the absorption of uranium from sulfate solution containing uranium by strong basic anionic resin Amberlite IRA-402 has been investigated. the purpose of this study is to investigate the effect of pH parameters, the amount of adsorbent used, the initial concentration of uranium metal ions and contact time on the amount of uranium absorption from the solution obtained from the leaching of the ore in the batch system. The results obtained for uranium absorption showed that at pH 3, the amount of adsorbent used is 2g/l and the equilibrium time is 100 minutes, the maximum amount of absorption occurs. In the study of the effect of concentration on uranium absorption, it was observed that with the increase of the initial concentration of metal ions, the absorption percentage decreases, but the absorption rate per gram unit of the adsorbent increases. The results of kinetic experiments in optimal conditions for uranium absorption and matching the experimental data with the first-order and second-order kinetic models showed that the process of uranium absorption by Amberlite IRA-402 resin follows the pseudo-second-order kinetic model.

RADIATION PROTECTION AND DOSIMETRY

Experimental study of the thermoluminescence response of the display screen of mobile phones for accident dosimetry

Articles in Press, Accepted Manuscript, Available Online from 24 November 2024

https://doi.org/10.24200/nst.2024.1677.2056

Amir Moslehi; Saeed Bagheri; Firouz Payervand

Abstract In this work, display screen samples of five mobile phone models including Huawei-y7, Nokia6, Iphone5, Sony-c3 and Shiaomi-note were investigated in order to use for accident dosimetry. After separation and washing with HF acid and ethanol, pieces with dimensions smaller than 5 mm × 5 mm from each sample were prepared. The samples were irradiated with 60Co gamma rays of Theratron 780 irradiator with a few absorbed doses between 0.01 and 10 Gy. Thermoluminescence (TL) signal of each sample normalized to its mass was measured with a Harshaw 4500 reader from 50 to 300 oC with a rate of 5 oC s-1. Calibration curves obtained for the samples showed that for all models the signal intensity linearly increases with the dose. On the other hand, significant light and time fading were observed for the TL signals measured for all models. Therefore, it is necessary to investigate the samples in darkness as soon as possible after the accident. Overall, Iphone5 possessing the most signal intensity per unit absorbed dose and the least minimum measurable dose (MMD) value recognized as the most appropriate model for accident dosimetry between the models investigated.

NUCLEAR FUEL CYCLE AND FUEL MATERIALS

Safety assessment of the fuel assembly drop accident in the core of Tehran Research Reactor (2)

Articles in Press, Accepted Manuscript, Available Online from 08 October 2024

https://doi.org/10.24200/nst.2024.1611.2040

Bahareh Roostaii; Behrouz Rokrok

Abstract In this research, a drop accident for a fuel assembly in Tehran research reactor on other fuel assembles inside the reactor core is analyzed mechanically during fuel shuffling or loading. The purpose of the analysis is to ensure the structural integrity of fuel assembly during this incident. In this simulation, the ABAQUS software is applied for collision analysis. Three modes are considered for a fuel assembly and its collision with another assembly inside the core. It includes the vertical and symmetrical impact of an assembly on top of another assembly; the second, vertical and asymmetric impact of an assembly on top of another assembly; and the third, vertical impact of an assembly of one assembly to the fuel side plate of another assembly in the reactor core. The stress analysis showed that in the first and second cases, the falling fuel assembly first hits the Handling Pin in the upper part of the target fuel assembly, and with its resilience, the fuel plate is protected against external impact force. But in the third case, the fuel side plates are damaged and there is a possibility of losing its integrity.

NUCLEAR PHYSICS AND RADIATION PHYSICS

Description of high-spin energy levels of 162Dy & 166Er nuclei by the three-level interaction boson model

Articles in Press, Accepted Manuscript, Available Online from 02 December 2024

https://doi.org/10.24200/nst.2024.1601.2035

Farzaneh Poursharif; hadi sabri; Saeedeh Akbari

Abstract In this paper, energy levels of the high-spin states of nuclei has been studied. To retrieving energy levels, the levels were first labeled based on the SU(3) dynamical limit of the interaction boson model and then the results were calculated in both the three-level and two-level interaction boson models. It can be seen that the developed three-level interaction boson model has a great advantage over the two-level model, and the spectrum obtained for energy levels using this model is in good agreement with the experimental spectrum, which shows that this model in the description and recovering energy levels with high spin state is more successful. This model also works better in describing levels of high spin states than . Examining the results of energy level calculations, it was observed that the developed three-level interaction boson model in retrieving the levels of nucleus is better than , because nucleus shows a higher degree of deformation than due to its deformation parameter value.

INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY

Evaluation of combined Compton-positron emission tomography imaging system to improve image quality using Monte Carlo simulation

Articles in Press, Accepted Manuscript, Available Online from 07 December 2024

https://doi.org/10.24200/nst.2024.1656.2049

F. Daei Ghafuri Basir; M. Gaffari; S.A. Hosseini

Abstract The combination of Compton imaging and positron emission tomography, which is also known as the combined Compton-positron emission tomography (Compton-PET) imaging system, has received attention due to the improvement of spatial resolution and imaging sensitivity compared to PET imaging alone. Compton-PET simulated system consists of two concentric detector rings. The inner ring with a smaller diameter is called the Compton scattering detector, the scatterer, and the outer ring, which has the dual use of Compton scattering detection and PET detector, is called the absorber. Considering the importance and many applications of PET imaging, the purpose of this research is to use the Compton-PET imaging approach and simulate this system with the 4GEANT tool, to achieve a better image output by increasing the spatial resolution. In this simulation, the geometry of two detector rings consisting of cubic crystals for the absorbing detector and the scattering detector inside the universe was considered. The gamma radiation source of the type that emits gamma with energy 511 keV was placed in the Micro-Derenzo phantom. In this research, image reconstruction is done using the MLEM iteration algorithm with 20 iterations. According to the obtained results, the value of FWHM is reported as 2.8 mm. For validation, the results were directly compared to the NEMA NU 2-2007 standard, which is provided for the measurement and reporting of positron emission tomography (PET) performance parameters.

INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY

Preparation of nitrobenzene-d5 from benzene-d6 with chemical purity and isotopic enrichment of 99.5%

Articles in Press, Accepted Manuscript, Available Online from 19 November 2024

https://doi.org/10.24200/nst.2024.1681.2059

Sodeh Sadjadi; elham mohagheghpour; Azadeh Haghshenas; Fahimeh Bayat

Abstract Substitution of hydrogen with deuterium as a heavier and stable isotope in different molecules leads to interesting and significant effects in various industries like electronics and medicine. One of the important applications of heavy water is the usage of it in hydrogen–deuterium exchange reactions for the production of organic compounds having deuterium atom. Deuterated nitrobenzene is a valuable raw material for the production of deuterated aniline used in organic light-emitting diode industries. The aim of this study is to consider the required conditions for the synthesis of nitrobenzene-d5 with 99.5% atom D. Our studies indicated that preparation of nitrobenzene-d5 from hydrogen–deuterium exchange is not an appropriate method. In this article, under the condition of nitration with sulfuric acid and nitric acid as a source of nitronium, nitrobenzene-d5 was synthesized from benzene-d6 produced from the reaction of benzene with heavy water. Reaction temperature and concentration of sulfuric acid and nitric acid were optimized in order to avoid by-product formation and also to prevent reduction in isotopic enrichment during the conversion of benzene-d6 to nitrobenzene-d5. The product was characterized and analyzed by FT-IR, 1HNMR, mass spectroscopy, and gas chromatography.

PLASMA PHYSICS AND FUSION THECHNOLOGY

Feasibility study of developing central-chord microwave interferometer of Alvand Tokamak to a multi-channel system

Articles in Press, Accepted Manuscript, Available Online from 09 July 2025

https://doi.org/10.24200/nst.2025.1742.2080

ehsanollah noori; mir mohammad reza seyedhabashi; Pouyan Samadifard

Abstract Microwave interferometers are among the most important diagnostic tools in measuring the electron density of tokamak plasma. However, single-channel interferometers only measure the linear average of the plasma density along the central chord of the tokamak cross-section and do not provide accurate information on the spatial distribution of the density. Multi-channel microwave interferometers allow for the measurement of the radial profile and spatial distribution of the tokamak plasma density. This information is essential for studying magnetic instabilities, optimizing energy transfer, and controlling the plasma. Currently, the interferometer in the Alvand tokamak is single-channel and only measures the linear average of the plasma density along the central chord. This limitation reduces the accuracy and comprehensiveness of the plasma data. The main objective of this paper is to design a multichannel interferometer system for the Alvand tokamak that can measure the radial profile and spatial distribution of electron density. This system is designed based on five symmetrical channels for transmitting and receiving microwave beams along the main radius and sub-chords of the Alvand tokamak to provide more comprehensive information on the spatial structure of the plasma. For efficient beam transmission with less loss, the use of tapered waveguides with larger dimensions was proposed. The requirements of spatial constraints for installing wave transmitting and receiving equipment around the vacuum chamber, measurement and calibration requirements of the proposed multi-channel interferometer were also examined. The proposed design will provide a significant improvement towards completing the active remote diagnostic systems of the Alvand Tokamak.

NUCLEAR PHYSICS AND RADIATION PHYSICS

Calculation of the level density and the level density parameter by taking into account the effect of statistical and quantum fluctuations using the Lipkin-Nogami model

Articles in Press, Accepted Manuscript, Available Online from 07 July 2025

https://doi.org/10.24200/nst.2025.1747.2082

Khosrow Benam

Abstract One of the important methods for studying the structure of the nucleus is the thermodynamic description of the nucleus. Although the nucleus consists of a fermionic system with a few particles, it experiences thermal fluctuations in particle number. In this task, thermodynamic quantities such as the excitation energy, level density parameter, and nuclear level density have been calculated by taking into account temperature-dependent pairing correlation as well as the statistical and quantum fluctuations using the LN model. Furthermore, by putting the calculated level density parameter from the LN model into the level density relation derived from the BSFG model, the nuclear level density has been obtained using this approach. Finally, the computed level densities using the mentioned models have been compared with each other and with the experimental level density.

NUCLEAR FUEL CYCLE AND FUEL MATERIALS

Feasibility study of uranium leaching from refractory ore

Articles in Press, Accepted Manuscript, Available Online from 21 October 2024

https://doi.org/10.24200/nst.2024.1680.2058

davood ghoddocy nejad

Abstract In this research, the recovery of uranium from refractory ores in the northern region of Isfahan by acid washing and acid leaching processes has been studied. Also, the effect of different parameters on acid washing and acid leaching was investigated. The results showed that acid concentration and liquid-to-solid ratio in acid washing as effective factors uof acid washing, as well as leaching temperature, leaching time, amount of acid and liquid-to-solid ratio are important factors in uranium recovery from refractory ores. The optimal parameters of the process include acid concentration of 0.5 M and liquid to solid ratio of 4.5 in the acid washing process, as well as temperature of 20 degrees Celsius, time of 5.5 hours, acid amount of 300 kg per ton of ore and ratio 2.5 liquid to solid was obtained in the sales process. Under these conditions, the efficiency of uranium extraction from refractory ores in the northern region of Isfahan was 83%.

INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY

Optimization and Evaluation of PMTs Arrangement in Large Plastic Scintillators for Position-Sensitive Detectors Using Geant4

Articles in Press, Accepted Manuscript, Available Online from 07 January 2025

https://doi.org/10.24200/nst.2025.1728.2074

javad kochakpour; Seyed Abolfazl Hosseini; Ali Taheri; Mojtaba Askari

Abstract This study focuses on evaluating and optimizing the arrangement of photomultiplier tubes (PMTs) in a plate plastic scintillator detector for applications in position-sensitive detection of radioactive sources. To achieve this, scintillation light processes within the detector were modeled and analyzed using Monte Carlo simulations implemented in the Geant4 toolkit. The research examines three distinct PMT configurations: a central configuration (PMTs placed at the center of each side of the detector), an asymmetric configuration (PMTs arranged unevenly with varying distances across the detector surface), and a corner configuration (PMTs positioned at the corners of the detector). Statistical analysis of the results indicates that the central configuration yields the best performance, with minimal errors: RMSE = 1.51 cm, MAE = 1.26 cm, MRE = 7.03%, and a correlation coefficient R = 0.997. In comparison, the second and third configurations demonstrate reduced accuracy in source localization. These findings suggest that an optimized PMT configuration can significantly enhance the precision and efficiency of detection systems, making them particularly effective for spatially sensitive applications in identifying and localizing radioactive sources.

RADIOLOGY AND NUCLEAR MEDICINE

Preparation and quality control of 225Ac-PSMA-617 with potential to treat prostate cancer

Articles in Press, Accepted Manuscript, Available Online from 12 January 2025

https://doi.org/10.24200/nst.2025.1707.2065

Fatemeh Rezazadeh-Sefideh; simindokht shirvani; Seyed Abolfazl Hosseini; Samaneh Zolghadri; Hassan Yousefnia; ali bahramisamani

Abstract Prostate-Specific Membrane Antigen (PSMA) is a membrane-bound glycoprotein that is overexpressed in prostate cancer. PSMA has been recognized as a promising target in the diagnosis and treatment of prostate cancer. Alpha particle-emitting radionuclides have shown promising results as radiotherapeutic agents for the treatment of metastatic castration-resistant prostate cancer (mCRPC). Actinium-225 (225Ac), with T½ = 9.9 d, has been one of the most commonly used options for clinical applications. 225Ac emits five alpha particles with energy ranges from 5.8 to 8.4 MeV during its decay chain. The decay cascade also includes beta particle emissions ranging from 0.6 to 2 MeV and gamma emissions from Francium-221 (221Fr) and Bismuth-213 (213Bi). Considering the favorable properties of this radionuclide for targeted alpha therapy of prostate cancer, this study initially determined the radionuclide purity of 225Ac using gamma spectrometry equipped with a high-resolution high-purity germanium detector and a liquid scintillation detector. Then, PSMA-617 labeling was performed with 225Ac at 95°C for 30 minutes. The radiochemical purity of the resulting compound was determined to be over %96 using thin-layer chromatography. This study demonstrated the successful labeling of PSMA-617 with 225Ac under optimal conditions and high radiochemical purity for clinical applications.

RADIOLOGY AND NUCLEAR MEDICINE

Calculating S values of the 225Ac decay chain using MCNP simulating code

Articles in Press, Accepted Manuscript, Available Online from 20 May 2025

https://doi.org/10.24200/nst.2025.1769.2091

Fatemeh Rezazadeh-Sefideh; Seyed Abolfazl Hosseini; simindokht shirvani; Samaneh Zolghadri; Hassan Yousefnia; Ali Bahrami-Samani

Abstract Among alpha-emitting radioactive nuclei for clinical applications, Actinium-225 (²²⁵Ac), with a half-life of 9.9 days, is widely used. This radionuclide undergoes a decay chain, emitting five alpha particles in the energy range of 5.8 to 8.4 MeV. The decay cascade also includes beta emissions from 0.6 to 2 MeV and gamma radiation from Francium-221 (²²¹Fr) and Bismuth-213 (²¹³Bi). This study aimed to calculate S-values, the absorbed dose per decay from the source organ to the target organ in mSv/MBq.s, for ²²⁵Ac and its daughters in the adult male ORNL phantom (225 source-target organ pairs) using the MCNPX2.7 code. The accuracy of the code was verified by computing the specific absorbed fraction (SAF) and comparing it with ORNL data. The results of MCNP and ORNL data showed strong agreement when the source-target organ distance and size were appropriate. However, in cases with greater distances or complex geometries, discrepancies were observed, attributed to the different computational methods used by ORNL in these situations. This study confirmed that ²²⁵Ac and its daughters, especially Polonium-213 (²¹³Po), deliver a high dose to target organs. The MCNPX simulation showed good accuracy compared to ORNL data and can aid in optimizing targeted alpha therapy.

MATERIALS SCIENCE

Investigation of coil deformation and metallurgical variations at the interface of dissimilar Aluminum-Copper Joints in magnetic pulse welding using Single-Sided and double-sided coil

Articles in Press, Accepted Manuscript, Available Online from 24 May 2025

https://doi.org/10.24200/nst.2025.1791.2102

Morteza Sarvari

Abstract In this study, magnetic pulse welding (MPW) is proposed as a solid-state welding solution for the metallurgical joining of dissimilar aluminum-copper metals. The coil type used in MPW is a critical factor influencing joint quality, depending on its geometry and electromagnetic performance. Two types of flat coil, a double-sided H-shaped coil and a single-sided E-shaped coil, were used for welding dissimilar aluminum-copper metals. Welding was performed at a discharge voltage of 16 kV, a capacitor bank of 120 μF, and an air gap of 0.7 mm. After 10 welding repetitions, the coils’ morphology was evaluated. The joint interface was analyzed using field emission scanning electron microscopy (FE-SEM). Examination of the coils showed that the double-sided inductor underwent plastic deformation after 10 welds due to magnetic field interference. This deformation increased the coil-workpiece gap, reducing process repeatability.The results of the electron microscope examination of the joint interface showed the formation of a transition zone, a wavy morphology, waves, and separated copper pieces at the joint interface. The formation of the transition zone occurred only in welding with a double-sided coil, which indicates a much higher impact intensity in the type of coil compared to the single-sided coil. Also, the width of the joint interface in welding using a single-sided coil has decreased from 3.5 μm to 0.6 μm compared to the double-sided coil.

NANO SCIENCE AND NANOTECHNOLOGY

Investigating the Effect of Magnetic Field on Nanoparticle Dose Enhancement in Protontherapy: Comparison of Single-stage and Phase-space Simulation Approaches

Articles in Press, Accepted Manuscript, Available Online from 25 May 2025

https://doi.org/10.24200/nst.2025.1793.2104

Jafar Alamgir; Seyed Abolfazl Hosseini,; ehsan salimi

Abstract Recently, special attention has been paid to the use of nanoparticles (NPs) in radiation therapy to enhance the therapeutic gain. Combining proton therapy with Magnetic Resonance Imaging has been developing rapidly. One of the associated challenges is the possible impact of a magnetic field on the dose distribution around NPs. In the present study, the dose enhancement factor of a 25 nm radius gold, gadolinium, and superparamagnetic iron oxide NP irradiated by protons of 50, 150, and 250 MeV has been examined with and without the presence of a static magnetic field with different strengths. In addition, two simulation approaches (single-stage and phase-space approaches) using the Geant4 toolkit are considered and the results from two electromagnetic physical lists, Livermore and Penelope, are compared. The results show that using heavier NPs (i.e., high density and effective atomic number) increases the dose more than the lighter ones. The difference between the two investigated physics lists is significant in the low-energy region and reaches up to 20% in dose enhancement factor calculations. Moreover, a magnetic field with a strength of up to 7 T did not reveal a significant effect on the dose distribution around NPs and the number of secondary particles. The results of this study have paved the way for experimental studies of the feasibility of combining proton therapy with the simultaneous presence of NPs and magnetic field, which can be helpful before the start of the clinical phase.

INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY

Investigation of the Behavior of Plate and Rod Plastic Scintillator Detectors in Source Positioning Based on Energy Spectrum Analysis

Articles in Press, Accepted Manuscript, Available Online from 08 June 2025

https://doi.org/10.24200/nst.2025.1790.2101

javad kochakpour; Seyed Abolfazl Hosseini,; Ali Taheri; Mojtaba Askari

Abstract Abstract: The aim of this study is to analyze and compare the spectral and spatial characteristics of plastic rod and plate detectors. In this context, the variations in the FWHM at the Compton edge of the energy spectrum at different source positions for both types of detectors were investigated. For this purpose, the energy spectra of the detectors were recorded at various source positions and analyzed separately. The dimensions of the rod detector were 5 × 50 cm, and the dimensions of the plate detector were 50 × 5 × 50 cm. The results show that as the distance between the source and the detector increases, the FWHM increases in both types of detectors; however, the change is more pronounced in the rod detector compared to the plate one. These differences are attributed to the geometric characteristics and photon scattering behavior in each detector. Furthermore, the results indicate that the rod detector have higher spatial resolution. These features could be useful in optimizing the geometric design of detectors for applications such as nuclear imaging, industrial tomography, and others.

NUCLEAR FUEL CYCLE AND FUEL MATERIALS

Investigation of the Effect of Top-End Pressure on Rotor Axial Pressure in a Gas Centrifuge Machine Using the DSMC Method

Articles in Press, Accepted Manuscript, Available Online from 03 August 2025

https://doi.org/10.24200/nst.2025.1801.2109

Sadegh Yousefi-Nasab; Jaber Safdari; Javad Karimi-Sabet

Abstract In centrifuge machines, the study of gas dynamics is of critical importance not only within the rotor but also in the surrounding external region. To reduce both pressure and frictional power losses in the space around the rotor, molecular pumps are employed. Given the direct interaction between the pressure in the top-end region and that within the rotor, understanding their mutual influence is essential for optimal machine design. Predicting the wall pressure of the rotor during the gas feed process, along with defining acceptable ranges for variations in operational and geometrical parameters that affect rotor axis pressure, is vital for maintaining stable pressure in the top-end region. These considerations underscore the importance of assessing how top-end pressure is influenced by rotor axis pressure. However, despite its significance for designers, direct measurement of rotor axis pressure faces substantial technical challenges. In this study, to establish the relationship between top-end pressure and rotor axis pressure, the gas flow within the entire external space of the rotor, as well as part of its internal region, was simulated using the Direct Simulation Monte Carlo (DSMC) method. Simulation results reveal that the pressure distribution inside and outside the rotor depends on the type of gas. Moreover, a correlation was derived showing that a 2.5-fold increase in top-end pressure results in a 70% rise in rotor axis pressure, while a tenfold increase in top-end pressure leads to an approximately threefold increase in rotor axis pressure.

RADIOLOGY AND NUCLEAR MEDICINE

Evaluation of the performance of parallel-hole collimators in response to different emission energies in SPECT imaging and optimization of their characteristics for high energies

Articles in Press, Accepted Manuscript, Available Online from 05 August 2025

https://doi.org/10.24200/nst.2025.1782.2096

Mahsa Noori-Asl; Maryam Ehtemali; Mohammad Hamdipour

Abstract One of the most important factors affecting the quality of images obtained from a SPECT imaging system is the physical characteristics of the collimator used. The aim of this study is to investigate the different components of the response of existing parallel-hole collimators (geometric, penetration, and scattering components) to the emission energies used in nuclear medicine imaging, and also to optimize the collimator parameters to achieve the highest value of the geometric component for high energies. The results of this study show that, considering the contribution of the geometric component, for emission energies of 68, 93, 135, 140, 159, 161, and 171 keV, the low-energy collimators LEHR and LEGP, for energies of 185 keV and 245 keV, the medium-energy collimators MEGP, and for energy of 300 keV, the high-energy collimators HEGP have the necessary efficiency. In contrast, for energies of 364 keV and 511 keV, the geometric response of any of the existing collimators is not sufficient. Hence, optimization of the collimator parameters for these two energies is necessary. According to the optimization results, high-energy collimators with the same hole size of 0.25 cm, the distance between the holes of 0.225 cm and 0.35 cm, and the collimator thickness of 7 cm and 8 cm, with geometric components of about 80% and 60%, are proposed as optimal collimators for energies of 364 keV and 511 keV, respectively.

NUCLEAR FUEL CYCLE AND FUEL MATERIALS

Study of Local Mass Transfer Resistances in Uranium Transport Using Hollow Fiber Liquid Membranes and Evaluation of Its Separation from Leaching Solutions

Articles in Press, Accepted Manuscript, Available Online from 06 September 2025

https://doi.org/10.24200/nst.2025.1861.2119

Fazel Zahakifar; Amir Charkhi; Meisam Torab-Mostaedi; Reza Davarkhah; Fereshte Khanramaki

Abstract In this study, uranium transport from a sulfate aqueous solution to an ammonium chloride solution was investigated using a hollow fiber liquid membrane (HFLM) unit containing Alamine 336. By applying different flow rates to the fiber lumen and the shell side of the hollow fiber liquid membrane module, uranium transport was examined, and the local mass transfer coefficients and resistances were calculated using the proposed empirical correlations. Through the simultaneous fitting of the obtained experimental data, the mass transfer equation coefficients were determined in terms of dimensionless numbers. The results indicated that the data fitting error was less than 6%. A comparison of the mass transfer resistances in the renewal layer, liquid membrane, and shell side revealed that uranium transport through the renewal layer is the rate-limiting step in the renewal-type hollow fiber liquid membrane system. The effect of the lumen flow rate on uranium separation from a real sample was also examined. Due to the reduction in the renewal layer thickness with increasing flow rate, uranium transport was enhanced. The results demonstrated that the hollow fiber liquid membrane consistently exhibited an efficient performance for uranium separation from real solutions. Moreover, with increasing flow rate, uranium separation from iron improves due to kinetic effects.

INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY

Quantum entanglement in the structure of Tellurium atomic nuclei within IBM-2 model

Articles in Press, Accepted Manuscript, Available Online from 07 September 2025

https://doi.org/10.24200/nst.2025.1857.2116

maryam ghapanvari; narjes amiri; masoud sayedi

Abstract This research examines the Quantum Phase Transition (QPT) between spherical even-even nuclei (U(5) ) up to the critical point E(5), which has been studied using entanglement entropy in the framework of the Interacting Boson Model 2 (IBM-2). To evaluate this observable, the Tellurium isotopic chain (Te ) has been chosen. The results indicated that the entanglement entropy in the region of U(5)-SO(6) has an increasing trend. Therefore, it is predicted that the isotopes Te(116) and Te(124) are suitable candidates for the symmetry limit U(5) and the critical point E(5), respectively . And the results we obtained from this research are in very good agreement with experimental data and other studies.

The simulation of dose variation effects due to the presence of different metal nanoparticles under proton irradiation using Geant4 toolkit

Volume 45, Issue 2, June 2024, Pages 54-64

https://doi.org/10.24200/nst.2024.1574

J. Alamgir; S.A. Hosseini; E. Salimi

Abstract The impacts of nanoparticles in radiation therapy have been investigated for many years now. The present study was conducted to investigate the effect of different physical interaction models on dose calculations using gold, hafnium and gadolinium nanoparticles. A nanoparticle with a diameter of 50 nm was simulated in a cubic water phantom. It was irradiated by protons with energies of 5, 50 and 150 MeV using Geant4 Monte Carlo toolkit. The current study considers various parameters, including the energy spectrum of secondary electrons and photons, radial dose distribution (RDD), dose enhancement factor (DEF), around the nanoparticle with three different materials and two physical interaction models. The obtained data showed that for gold nanoparticles, the Penelope model generated a greater number of secondary electrons than the Livermore model; however, for the other two nanoparticles, the Livermore model produced a greater number of secondary electrons than the Penelope model. In the RDD graphs, the Penelope model presents a 10% difference compared to the Livermore model up to a distance of 6 nm from the nanoparticle’s surface (along the radial axis in water). Furthermore, the Livermore model indicates a 16% and 10% increase in dose compared to the Penelope model. This is up to a distance of 9 nm from the surface of hafnium and gadolinium nanoparticles, respectively. In the case of DEF, the dose deposited around the gold nanoparticle was increased by 14. This is the highest amount in comparison to DEF of hafnium and gadolinium nanoparticles which is 10 and 6, respectively.

Investigation of electron beam irradiation effect on spikes of SARS-COV2, MERS-COV, UK variant, SARS-COV by Geant4-DNA toolkit

Volume 44, Issue 2, June 2023, Pages 38-46

https://doi.org/10.24200/nst.2022.1003.1680

M. Jalili Torkamani; F. Zolfagharpour; A. Asadi; P. Sayyahkoohi

Abstract Viruses pass cell walls and enter cells using their spikes, So one of the efficient ways to stop viral infections is to disturb their spikes functionality. In this research, the process of energy absorption and transfer by SARS-COV2, MERS-COV, UK-COV, and SARS-COV spikes was studied. In this research sample viruses exposed to radioactive radiations and results were compared by Geant4-DNA and analyzed. A strategy to reduce the virus life cycle is energy absorption. In this research, the response to viruses spikes to radiation was simulated. Samples were exposed to 10 eV–2 keV electron beams. The level of Energy absorption and its relation to the number of infected patients was studied. It was concluded there is an inverse relationship between absorbed energy level and patient death.

The importance of a closed fuel cycle in achieving sustainable and renewable nuclear energy in Iran

Volume 46, Issue 1, April 2025, Pages 176-187

https://doi.org/10.24200/nst.2024.1533.2000

M. Ghorbani Ashraf; P. Hatami Barough

Abstract Energy security is one of the most important factors in the sustainable development of societies. Fulfillment of goals such as economic development, increasing social well-being, and improving the quality of life depend on providing energy and guaranteeing stable and reliable, clean, and affordable resources. In recent years, the use of renewable resources has received a lot of attention to diversify their energy portfolio, reduce the harmful effects on the environment, and achieve sustainable energy. From this point of view, with the proper establishment of the nuclear fuel cycle, nuclear energy can be considered as renewable and sustainable energy in the energy portfolio and compensate for the lack of non-renewable energy in the future. The purpose of this paper is to explain the importance of a closed fuel cycle in achieving sustainable and renewable nuclear energy. Also, due to the not-very favorable situation of uranium and thorium resources in Iran, the lack of extensive international cooperation, the existence of sanctions in the provision of raw materials for nuclear fuel production, and the impossibility of guaranteeing the supply of fuel needed for nuclear energy production, the need to pay more attention to establishing a closed fuel cycle and using fast breeder reactors is proven. Paying attention to this important issue will achieve goals such as reducing the need for natural uranium, reducing the cost of nuclear waste, improving the efficiency of nuclear power plants, and producing materials required for the use of radiation in industry, medicine, and health.

A study on the use of swarm robotics for environmental monitoring, radiation mapping and the discovery of radioactive sources

Volume 46, Issue 1, April 2025, Pages 136-147

https://doi.org/10.24200/nst.2024.1628

H. Ardiny; A.M. Beigzadeh

Abstract Exploring and mapping radioactive environments presents potentially challenging and risky tasks. To ensure safety, the use of robots can help mitigate these risks. However, deploying a single robot may not be enough to effectively cover the entire area. Therefore, the technique of using multiple robots or a robot swarm can play a significant role in reducing time and improving the exploration and mapping process. Additionally, multi-robot systems have high reliability, and if a number of robots fail due to reasons such as radiation exposure, the remaining robots can continue the mission. This article focuses on the use of several autonomous robots simultaneously for radiation mapping and the discovery of radioactive sources. The study has examined various approaches, including the effect of the number and absorbed dose of robots. The results indicate that increasing the number of robots can enhance the speed of exploration, but the rate of increase is lower than the rate of the robot number due to the crowding of robots. To achieve optimal exploration, it is necessary to utilize more advanced models, such as movement patterns inspired by nature. This paper presents valuable insights into the coordination of collective robots for searching in radioactive environments, which could open up opportunities for the application of swarm intelligence in nuclear scenarios.

Monte Carlo simulation of IECF using Geant4 for neutron radiography

Volume 44, Issue 2, June 2023, Pages 22-29

https://doi.org/10.24200/nst.2023.1368

S. Vosoughi; P. Rafiepour; M. Mehrabi; M. Ghapanvari; N. Salek

Abstract Neutron radiography (NRG) is a non-destructive imaging technique for image generation using neutron radiation. In this paper, feasibility studies of neutron radiography for IECF were performed by Geant4 Monte Carlo code. The effects of the different thicknesses of lead on the image and the detection possibility of cavities with different sizes inside a thick lead have been investigated to understand the performance of the device for neutron radiography purposes. The quality of the images was evaluated in terms of contrast. The simulation results showed the efficiency and limitations of NRG for IECF devices and the potential areas where NRG can be performed.

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